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Article Dans Une Revue Current Opinion in Electrochemistry Année : 2022

Microstructurally resolved modeling of all solid-state batteries: Latest progresses, opportunities, and challenges

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Résumé

All solid-state batteries are promising high-energy-density storage devices. To optimize their performance without costly trial and error approaches, microstructure-resolved continuum models have been proposed to understand the influence of the electrode architecture on their capabilities. We discuss the recent advances in the microstructure-resolved modeling of solid-state batteries. While not all of the experimentally observed phenomena can be accurately represented, these models generally agree that the low ionic conductivity of the solid electrolyte is a limiting factor. We conclude by highlighting the need for microstructure-resolved models of degradation mechanisms, manufacturing effects and artificial intelligence approaches speeding up the optimization of interfaces in all solid-state-battery electrodes.

Domaines

Chimie Matériaux

Dates et versions

hal-03880347 , version 1 (01-12-2022)

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Citer

Mohammed Alabdali, Franco Zanotto, Virginie Viallet, Vincent Seznec, Alejandro Franco. Microstructurally resolved modeling of all solid-state batteries: Latest progresses, opportunities, and challenges. Current Opinion in Electrochemistry, 2022, 36, pp.101127. ⟨10.1016/j.coelec.2022.101127⟩. ⟨hal-03880347⟩
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